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Summary
"To mark ones self permanently is to propose true unity with the other. To be joined together as one, in the eyes of the Lord."
The day Castiel pulled Dean from the pit was the day his Grace claimed Dean's soul as his. Humans can't carry Grace and Angels can't have souls. So what's an Angel of the Lord to do when he has fallen in love with a hunter who gave him a piece of his soul? Fall all over again.
Dean gets a tattoo of Castiel's handprint and it causes their Grace/Soul bond to ignite inside them. Only two options are available. Either break the bond, remove the Grace and let the soul inside Castiel die away, thus turning him into a full fledged Angel with no recollection of Dean and no favor over him. Or use the Grace to bind their souls together for eternity and let Castiel fall from Heaven and Grace to become a human, to live out his life as a Hunter among the Winchester boys.
